Typically, /CS pin of Si534x/8x/9x SPI should be pulled up to be High (logic 1) between each two bytes transfer for reliability. In case of rare alignment issues, setting /CS high will help the SPI logic to recover by reinitializing its state machine. An example timing diagram of issuing the pulse of /CS is shown as below:
An example brief timing diagram of /CS pulse sequences is shown in the below figure. The left sequence is recommended for Si534x/8x/9x SPI; the right one may work to achieve several transfers of more than two bytes while /CS is kept as low. However, it is the responsibility of the user to test sufficiently to ensure SPI communication reliability.